TY - JOUR
T1 - Evolution of superconducting and normal state properties of Fe1.09Se0.55Te0.45 under pressure
AU - Krishnan, Manikandan
AU - Ishigaki, Kento
AU - Mariappan, Sathiskumar
AU - Sokkalingam, Rajkumar
AU - Gouchi, Jun
AU - Bhoi, Dilip
AU - Sankar, Raman
AU - Vajeeston, Ponniah
AU - Jing, Qiang
AU - Uwatoko, Yoshiya
AU - Liu, Bo
AU - Sonachalam, Arumugam
N1 - Publisher Copyright:
© 2025 Elsevier Ltd
PY - 2025/6
Y1 - 2025/6
N2 - The Fe1+ySe1-xTex family of iron-based superconductors are extensively investigated for their unconventional nature of superconductivity, which arises from a complex interplay of spin and orbital ordering. At ambient conditions, Fe1.09Se0.55Te0.45 exhibits a superconducting transition below Tc∼14 K and a nematic ordering accompanied by a tetragonal to orthorhombic structural change at (Ts) which is marked by a sign change of Hall coefficient (RH) from positive to negative. In addition, the normal state resistivity follows a -log(T) increase with decreasing temperature due to the presence of excess Fe impurity acting as Kondo scattering centre. In this work, we investigate the evolution of superconducting and normal state properties of Fe1.09Se0.55Te0.45, a member of the Fe1+ySe1-xTex family, under hydrostatic pressure (P) using magneto-transport, dc magnetization and complementary first-principles band structure calculations. With applied P, the superconducting Tc reveals a dome-like shape, reaching a maximum Tc ∼19.9 K at critical pressure Pc ∼3.3 GPa. Simultaneously, with increasing pressure, both the -log(T) resistivity increase and Ts are gradually suppressed. Near Pc, Ts almost disappears, while the -log(T) resistivity increase persist beyond Pc up to 5 GPa and a Fermi liquid like behaviour emerges around 8 GPa. Furthermore, the band structure calculations suggest a pressure-induced structural change from orthorhombic to monoclinic symmetry near Pc. The nontrivial nature is evidenced by the effects of high pressure on the charge carrier balance, phase transition and superconductivity in Fe1.09Se0.55Te0.45. This nontrivial superconductivity is strongly linked to the significant normal state that arises from the connection between Fermi surface reconstruction and structural phase transitions.
AB - The Fe1+ySe1-xTex family of iron-based superconductors are extensively investigated for their unconventional nature of superconductivity, which arises from a complex interplay of spin and orbital ordering. At ambient conditions, Fe1.09Se0.55Te0.45 exhibits a superconducting transition below Tc∼14 K and a nematic ordering accompanied by a tetragonal to orthorhombic structural change at (Ts) which is marked by a sign change of Hall coefficient (RH) from positive to negative. In addition, the normal state resistivity follows a -log(T) increase with decreasing temperature due to the presence of excess Fe impurity acting as Kondo scattering centre. In this work, we investigate the evolution of superconducting and normal state properties of Fe1.09Se0.55Te0.45, a member of the Fe1+ySe1-xTex family, under hydrostatic pressure (P) using magneto-transport, dc magnetization and complementary first-principles band structure calculations. With applied P, the superconducting Tc reveals a dome-like shape, reaching a maximum Tc ∼19.9 K at critical pressure Pc ∼3.3 GPa. Simultaneously, with increasing pressure, both the -log(T) resistivity increase and Ts are gradually suppressed. Near Pc, Ts almost disappears, while the -log(T) resistivity increase persist beyond Pc up to 5 GPa and a Fermi liquid like behaviour emerges around 8 GPa. Furthermore, the band structure calculations suggest a pressure-induced structural change from orthorhombic to monoclinic symmetry near Pc. The nontrivial nature is evidenced by the effects of high pressure on the charge carrier balance, phase transition and superconductivity in Fe1.09Se0.55Te0.45. This nontrivial superconductivity is strongly linked to the significant normal state that arises from the connection between Fermi surface reconstruction and structural phase transitions.
KW - Fermi surface reconstruction
KW - High pressure
KW - Kondo scattering
KW - Nematic phase transition
KW - Superconductivity
UR - http://www.scopus.com/inward/record.url?scp=85218997211&partnerID=8YFLogxK
U2 - 10.1016/j.jpcs.2025.112628
DO - 10.1016/j.jpcs.2025.112628
M3 - Article
AN - SCOPUS:85218997211
SN - 0022-3697
VL - 201
JO - Journal of Physics and Chemistry of Solids
JF - Journal of Physics and Chemistry of Solids
M1 - 112628
ER -